It is a bit ambiguous in this case.
The anime finished before the manga:
Anime finished: December 18, 2011
Manga finished: June 26, 2013
MangaUpdates contains information about the anime adaptation and indicates that it is complete.
Here you have all the anime relations we detected ordered by release date, so you can see the reason for this status in context and also use it as watching order.
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Anime - Base
Release date: October 02, 2011
Maji de Watashi ni Koi Shinasai! is set in a town steeped in samurai tradition, focusing on a group of close-knit high school friends at Kawakami Academy.
These students are known for embodying the values of samurai, striving for excellence in their studies, sports, and preservation of their heritage.
The story revolves around Yamato Naoe and his six friends, a balanced group of three boys and three girls who support and challenge each other.
However, their dynamic is disrupted by the arrival of two new girls, adding complexity and potential romantic interests into their already established group.
The anime explores how they navigate these changes while maintaining their commitment to samurai ideals and facing the challenges of adolescence and newfound feelings.